吸附法处理氨氮废水研究进展
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摘要
简介了常用的吸附氨氮材料——沸石、生物质炭、膨润土、粉煤灰等在吸附功能上的优缺点;分析了氨氮吸附材料吸附去除废水中氨氮的作用机制;阐述了国内外不同吸附材料吸附氨氮的研究进展;比较了不同吸附材料及不同改性方法在氨氮去除率和氨氮吸附量上的区别;展望了吸附法去除废水中氨氮的未来研究方向;吸附法去除废水中氨氮的机理及相关的应用研究还有待进一步研究。
The merits and demerits of various kinds of commonly used ammonia nitrogen adsorption materials——biomass carbon,bentonite and fly ash,are briefly introduced; The mechanism of adsorption removal of ammonia nitrogen from wastewater by ammonia nitrogen adsorption was analyzed; The research progress of adsorption of ammonia nitrogen by different adsorbent materials at home and abroad was described; The differences between different adsorbent materials and different modification methods in removal rate and adsorption amount of ammonia nitrogen were compared; The future research direction of adsorption removal of ammonia nitrogen from wastewater is prospected; The mechanism and related application of adsorption method to remove ammonia nitrogen from wastewater need further study.
The merits and demerits of various kinds of commonly used ammonia nitrogen adsorption materials——biomass carbon,bentonite and fly ash,are briefly introduced; The mechanism of adsorption removal of ammonia nitrogen from wastewater by ammonia nitrogen adsorption was analyzed; The research progress of adsorption of ammonia nitrogen by different adsorbent materials at home and abroad was described; The differences between different adsorbent materials and different modification methods in removal rate and adsorption amount of ammonia nitrogen were compared; The future research direction of adsorption removal of ammonia nitrogen from wastewater is prospected; The mechanism and related application of adsorption method to remove ammonia nitrogen from wastewater need further study.
引文
[1] Shu J,Liu R,Liu Z,et al. Simultaneous removal of ammonia nitrogen and manganese from wastewater using nitrite by electrochemical method[J]. Environmental Technology Letters,2017,38(3):370-376.
[2] Wang H,Zhou Q,Zhang G,et al. A novel PSB-EDI system for high ammonia wastewater treatment,biomass production and nitrogen resource recovery:PSB system[J]. Water Science&Technology A Journal of the International Association on Water Pollution Research,2016,74(3):616-624.
[3]鲁秀国,杨凌焱,黄林长,等.非粮生物质吸附剂吸附水中氨氮的研究进展[J].华东交通大学学报,2018,35(1):90-95.
[4] Zhu L,Dong D,Hua X,et al. Ammonia nitrogen removal and recovery from acetylene purification wastewater by air stripping[J]. Water Science&Technology A Journal of the International Association on Water Pollution Research,2017,75(11):2538-2545.
[5] Kumar R,Pal P. Assessing the feasibility of N and P recovery by struvite precipitation from nutrient-rich wastewater:a review[J]. Environmental Science&Pollution Research International,2015,22(22):17453-17464.
[6]郭琳,刘晨,吴叶,等. MgO催化臭氧氧化水中氨氮的研究[J].工业水处理,2017,37(6):48-51.
[7] Shao Y,Shi Y,Mohammed A,et al. Wastewater ammonia removal using an integrated fixed-film activated sludge-sequencing batch biofilm reactor(IFAS-SBR):Comparison of suspended flocs and attached biofilm[J]. International Biodeterioration&Biodegradation,2017,116:38-47.
[8] Bhavsar K,Shah N K,Buha D,et al. Kinetic and equilibrium isotherm studies of ammoniacal nitrogen adsorption onto sugarcane bagasse from wastewater[J]. Desalination&Water Treatment,2017,60:180-187.
[9]罗宇智,沈明伟,李博.化学沉淀——折点氯化法处理稀土氨氮废水[J].有色金属(冶炼部分),2015(7):63-65.
[10] Shu J,Liu R,Liu Z,et al. Manganese recovery and ammonia nitrogen removal from simulation wastewater by pulse electrolysis[J]. Separation&Purification Technology,2016,168:107-113.
[11]唐朝春,叶鑫,陈惠民,等.地下水除铁除锰技术与应用的研究进展[J].华东交通大学学报,2016(1):136-142.
[12] Ding J,Zhao Q L,Zhang J,et al. Hybrid electrooxidation and adsorption process for the removal of ammonia in low concentration chloride wastewater[J]. Environmental Science&Pollution Research,2017,24(6):5098-5105.
[13] Chen Y,Wu Y,Liu C,et al. Low-temperature conversion of ammonia to nitrogen in water with ozone over composite metal oxide catalyst[J]. Journal of Environmental Sciences,2018,66:265-273.
[14] Ali I,Asim M,Khan T A. Low cost adsorbents for the removal of organic pollutants from wastewater[J]. Journal of Environmental Management,2012,113(1):170-183.
[15]郭俊元.微生物絮凝与改性沸石吸附联合处理猪场废水的研究[D].长沙:湖南大学,2013.
[16]张华.柚皮基活性炭制备及吸附应用机理研究[D].南宁:广西大学,2013.
[17] Xing Y,Xin-Qing L,Zhou Z H,et al. Adsorption and kinetics of ammonium from aqueous medium onto biochar[J]. Earth&Environment,2011,39(4):511-516.
[18] Liu N,Sun Z T,Wu Z C,et al. Adsorption characteristics of ammonium nitrogen by biochar from diverse origins in water[J]. Advanced Materials Research,2013,664:305-312.
[19] Kizito S,Wu S,Kipkemoi K W,et al. Evaluation of slow pyrolyzed wood and rice husks biochar for adsorption of ammonium nitrogen from piggery manure anaerobic digestate slurry[J]. Science of the Total Environment,2015,505:102-112.
[20] Zheng,Zeng,Song-da,et al. Sorption of ammonium and phosphate from aqueous solution by biochar derived from phytoremediation plants[J]. Journal of Zhejiang University Science B:Biomedicine&Biotechnology,2013,14(12):1152-1161.
[21] Tian M,Zeng Z,Jiang Z. Progress of preparation and applications of bamboo charcoal[J]. Materials Review,2015,29(1):143-146.
[22] Abdulrazzaq H,Jol H,Husni A,et al. Characterization and stabilisation of biochars obtained from empty fruit bunch,wood,and rice husk[J]. Bioresources,2014,9(2):2888-2898.
[23]崔凯.改性沸石处理废水中氨氮的研究[D].沈阳:沈阳工业大学,2016.
[24]许育新,喻曼,陈喜靖,等.天然沸石对水中氨氮吸附特性的研究[J].农业资源与环境学报,2015(3):250-256.
[25]王文超,管俊芳,严春杰,等.斜发沸石处理氨氮废水[J].环境工程学报,2014,8(3):1036-1040.
[26]王文超.片沸石颗粒吸附剂的制备及在氨氮废水处理中的应用[D].武汉:武汉理工大学,2014.
[27]陈吉吉,李日强.天然麦壳对氨氮吸附性能的研究[J].山西科技,2014,29(1):80-84.
[28]刘雪梅,陈嘉玮,王宇航.磷酸改性油茶壳活性炭吸附水中的氨氮研究[J].工业安全与环保,2018,44(2):11-14.
[29] Ibrahim A,Yusof L,Beddu N S,et al. Adsorption study of ammonia nitrogen by watermelon rind[C]. Bali:IOP Conference Series,2016.
[30]张广兴,邵红,李云娇,等.复合改性膨润土对氨氮废水的吸附及脱附[J].环境工程学报,2017(3):1494-1500.
[31]贾汉英,贺希格图,王继慧,等.改性粉煤灰吸附稀土氨氮废水的机理研究[J].有色金属(冶炼部分),2017(10):71-74.
[32]郭祎阁,赵颖,郭宇杰,等.壳聚糖包覆介孔微孔分子筛去除水中的氨氮[J].环境工程学报,2015,9(5):2067-2072.
[33] Couto R S,Oliveira A F,Guarino A W,et al. Removal of ammonia nitrogen from distilled old landfill leachate by adsorption on raw and modified aluminosilicate[J]. Environmental Technology,2017,38(7):816-826.
[34] Wei J,Liu X,Xu S. Adsorption behaviors of ammonium nitrogen by an amphoteric hydrogel[J]. Desalination&Water Treatment,2016,57(13):5753-5759.
[35]靳薛凯.片沸石对含氨废水的吸附研究[D].石家庄:河北科技大学,2017.
[36] Shirvani M,Kalbasi M,Shariatmadari H,et al. Sorptiondesorption of cadmium in aqueous palygorskite,sepiolite,and calcite suspensions:isotherm hysteresis[J]. Chemosphere,2006,65(11):2178-2184.
[37] Sancho I,Licon E,Valderrama C,et al. Recovery of ammonia from domestic wastewater effluents as liquid fertilizers by integration of natural zeolites and hollow fibre membrane contactors[J]. Science of the Total Environment,2017,s 584/585:244-251.
[38] Shaban M,Abukhadra M R,Nasief F M,et al. Removal of ammonia from aqueous solutions,ground water,and wastewater using mechanically activated clinoptilolite and synthetic zeolite-A:Kinetic and equilibrium studies[J].Water Air&Soil Pollution,2017,228(11):450-466.
[39]唐登勇,郑正,郭照冰,等.改性沸石吸附低浓度氨氮废水及其脱附的研究[J].环境工程学报,2011,5(2):293-296.
[40]饶力,汪晓军.天然沸石处理氨氮废水的中试研究[J].水处理技术,2016(4):104-106.
[41] Feiyue L,Yue X,Lei S,et al. Adsorption of ammonia nitrogen in wastewater using rice husk derived biochar[J]. Chinese Journal of Environmental Engineering,2015,9(3):1221-1226.
[42] Bhatnagar A,SillanpM,Witekkrowiak A. Agricultural waste peels as versatile biomass for water purification-a review[J]. Chemical Engineering Journal,2015,270:244-271.
[43]胡婧.吸附-介电泳法去除水中氨氮的工艺及机理研究[D].北京:中央民族大学,2015.
[44] Belhouchat N,Zaghouane-Boudiaf H,Viseras C. Removal of anionic and cationic dyes from aqueous solution with activated organo-bentonite/sodium alginate encapsulated beads[J]. Applied Clay Science,2017,135:9-15.
[45]刘丹.壳聚糖改性膨润土处理氨氮废水的实验研究[J].辽宁化工,2015(12):1423-1425.
[46]陈莉荣,李玉梅,杜明展.改性粉煤灰吸附稀土废水中的氨氮[J].环境工程学报,2013,7(2):518-522.
[47] Reitzel K,Andersen F,Egemose S,et al. Phosphate adsorption by lanthanum modified bentonite clay in fresh and brackish water[J]. Water Research,2013,47(8):2787-2796.
[48]刘志超,史晓燕,李艳根,等.镧改性粉煤灰及其脱氮除磷效果研究[J].化工新型材料,2018,46(2):205-208.
[49] Zhang Y,Yu F,Cheng W,et al. Adsorption equilibrium and kinetics of the removal of ammoniacal nitrogen by zeolite X/activated carbon composite synthesized from elutrilithe[J]. Journal of Chemistry,2017,2017(3):1-9.
[50] Chen Y Q,Tang J J,Wen-Long L I,et al. Thermal decomposition of magnesium ammonium phosphate and adsorption properties of its pyrolysis products toward ammonia nitrogen[J]. Transactions of Nonferrous Metals Society of China,2015,25(2):497-503.
[2] Wang H,Zhou Q,Zhang G,et al. A novel PSB-EDI system for high ammonia wastewater treatment,biomass production and nitrogen resource recovery:PSB system[J]. Water Science&Technology A Journal of the International Association on Water Pollution Research,2016,74(3):616-624.
[3]鲁秀国,杨凌焱,黄林长,等.非粮生物质吸附剂吸附水中氨氮的研究进展[J].华东交通大学学报,2018,35(1):90-95.
[4] Zhu L,Dong D,Hua X,et al. Ammonia nitrogen removal and recovery from acetylene purification wastewater by air stripping[J]. Water Science&Technology A Journal of the International Association on Water Pollution Research,2017,75(11):2538-2545.
[5] Kumar R,Pal P. Assessing the feasibility of N and P recovery by struvite precipitation from nutrient-rich wastewater:a review[J]. Environmental Science&Pollution Research International,2015,22(22):17453-17464.
[6]郭琳,刘晨,吴叶,等. MgO催化臭氧氧化水中氨氮的研究[J].工业水处理,2017,37(6):48-51.
[7] Shao Y,Shi Y,Mohammed A,et al. Wastewater ammonia removal using an integrated fixed-film activated sludge-sequencing batch biofilm reactor(IFAS-SBR):Comparison of suspended flocs and attached biofilm[J]. International Biodeterioration&Biodegradation,2017,116:38-47.
[8] Bhavsar K,Shah N K,Buha D,et al. Kinetic and equilibrium isotherm studies of ammoniacal nitrogen adsorption onto sugarcane bagasse from wastewater[J]. Desalination&Water Treatment,2017,60:180-187.
[9]罗宇智,沈明伟,李博.化学沉淀——折点氯化法处理稀土氨氮废水[J].有色金属(冶炼部分),2015(7):63-65.
[10] Shu J,Liu R,Liu Z,et al. Manganese recovery and ammonia nitrogen removal from simulation wastewater by pulse electrolysis[J]. Separation&Purification Technology,2016,168:107-113.
[11]唐朝春,叶鑫,陈惠民,等.地下水除铁除锰技术与应用的研究进展[J].华东交通大学学报,2016(1):136-142.
[12] Ding J,Zhao Q L,Zhang J,et al. Hybrid electrooxidation and adsorption process for the removal of ammonia in low concentration chloride wastewater[J]. Environmental Science&Pollution Research,2017,24(6):5098-5105.
[13] Chen Y,Wu Y,Liu C,et al. Low-temperature conversion of ammonia to nitrogen in water with ozone over composite metal oxide catalyst[J]. Journal of Environmental Sciences,2018,66:265-273.
[14] Ali I,Asim M,Khan T A. Low cost adsorbents for the removal of organic pollutants from wastewater[J]. Journal of Environmental Management,2012,113(1):170-183.
[15]郭俊元.微生物絮凝与改性沸石吸附联合处理猪场废水的研究[D].长沙:湖南大学,2013.
[16]张华.柚皮基活性炭制备及吸附应用机理研究[D].南宁:广西大学,2013.
[17] Xing Y,Xin-Qing L,Zhou Z H,et al. Adsorption and kinetics of ammonium from aqueous medium onto biochar[J]. Earth&Environment,2011,39(4):511-516.
[18] Liu N,Sun Z T,Wu Z C,et al. Adsorption characteristics of ammonium nitrogen by biochar from diverse origins in water[J]. Advanced Materials Research,2013,664:305-312.
[19] Kizito S,Wu S,Kipkemoi K W,et al. Evaluation of slow pyrolyzed wood and rice husks biochar for adsorption of ammonium nitrogen from piggery manure anaerobic digestate slurry[J]. Science of the Total Environment,2015,505:102-112.
[20] Zheng,Zeng,Song-da,et al. Sorption of ammonium and phosphate from aqueous solution by biochar derived from phytoremediation plants[J]. Journal of Zhejiang University Science B:Biomedicine&Biotechnology,2013,14(12):1152-1161.
[21] Tian M,Zeng Z,Jiang Z. Progress of preparation and applications of bamboo charcoal[J]. Materials Review,2015,29(1):143-146.
[22] Abdulrazzaq H,Jol H,Husni A,et al. Characterization and stabilisation of biochars obtained from empty fruit bunch,wood,and rice husk[J]. Bioresources,2014,9(2):2888-2898.
[23]崔凯.改性沸石处理废水中氨氮的研究[D].沈阳:沈阳工业大学,2016.
[24]许育新,喻曼,陈喜靖,等.天然沸石对水中氨氮吸附特性的研究[J].农业资源与环境学报,2015(3):250-256.
[25]王文超,管俊芳,严春杰,等.斜发沸石处理氨氮废水[J].环境工程学报,2014,8(3):1036-1040.
[26]王文超.片沸石颗粒吸附剂的制备及在氨氮废水处理中的应用[D].武汉:武汉理工大学,2014.
[27]陈吉吉,李日强.天然麦壳对氨氮吸附性能的研究[J].山西科技,2014,29(1):80-84.
[28]刘雪梅,陈嘉玮,王宇航.磷酸改性油茶壳活性炭吸附水中的氨氮研究[J].工业安全与环保,2018,44(2):11-14.
[29] Ibrahim A,Yusof L,Beddu N S,et al. Adsorption study of ammonia nitrogen by watermelon rind[C]. Bali:IOP Conference Series,2016.
[30]张广兴,邵红,李云娇,等.复合改性膨润土对氨氮废水的吸附及脱附[J].环境工程学报,2017(3):1494-1500.
[31]贾汉英,贺希格图,王继慧,等.改性粉煤灰吸附稀土氨氮废水的机理研究[J].有色金属(冶炼部分),2017(10):71-74.
[32]郭祎阁,赵颖,郭宇杰,等.壳聚糖包覆介孔微孔分子筛去除水中的氨氮[J].环境工程学报,2015,9(5):2067-2072.
[33] Couto R S,Oliveira A F,Guarino A W,et al. Removal of ammonia nitrogen from distilled old landfill leachate by adsorption on raw and modified aluminosilicate[J]. Environmental Technology,2017,38(7):816-826.
[34] Wei J,Liu X,Xu S. Adsorption behaviors of ammonium nitrogen by an amphoteric hydrogel[J]. Desalination&Water Treatment,2016,57(13):5753-5759.
[35]靳薛凯.片沸石对含氨废水的吸附研究[D].石家庄:河北科技大学,2017.
[36] Shirvani M,Kalbasi M,Shariatmadari H,et al. Sorptiondesorption of cadmium in aqueous palygorskite,sepiolite,and calcite suspensions:isotherm hysteresis[J]. Chemosphere,2006,65(11):2178-2184.
[37] Sancho I,Licon E,Valderrama C,et al. Recovery of ammonia from domestic wastewater effluents as liquid fertilizers by integration of natural zeolites and hollow fibre membrane contactors[J]. Science of the Total Environment,2017,s 584/585:244-251.
[38] Shaban M,Abukhadra M R,Nasief F M,et al. Removal of ammonia from aqueous solutions,ground water,and wastewater using mechanically activated clinoptilolite and synthetic zeolite-A:Kinetic and equilibrium studies[J].Water Air&Soil Pollution,2017,228(11):450-466.
[39]唐登勇,郑正,郭照冰,等.改性沸石吸附低浓度氨氮废水及其脱附的研究[J].环境工程学报,2011,5(2):293-296.
[40]饶力,汪晓军.天然沸石处理氨氮废水的中试研究[J].水处理技术,2016(4):104-106.
[41] Feiyue L,Yue X,Lei S,et al. Adsorption of ammonia nitrogen in wastewater using rice husk derived biochar[J]. Chinese Journal of Environmental Engineering,2015,9(3):1221-1226.
[42] Bhatnagar A,SillanpM,Witekkrowiak A. Agricultural waste peels as versatile biomass for water purification-a review[J]. Chemical Engineering Journal,2015,270:244-271.
[43]胡婧.吸附-介电泳法去除水中氨氮的工艺及机理研究[D].北京:中央民族大学,2015.
[44] Belhouchat N,Zaghouane-Boudiaf H,Viseras C. Removal of anionic and cationic dyes from aqueous solution with activated organo-bentonite/sodium alginate encapsulated beads[J]. Applied Clay Science,2017,135:9-15.
[45]刘丹.壳聚糖改性膨润土处理氨氮废水的实验研究[J].辽宁化工,2015(12):1423-1425.
[46]陈莉荣,李玉梅,杜明展.改性粉煤灰吸附稀土废水中的氨氮[J].环境工程学报,2013,7(2):518-522.
[47] Reitzel K,Andersen F,Egemose S,et al. Phosphate adsorption by lanthanum modified bentonite clay in fresh and brackish water[J]. Water Research,2013,47(8):2787-2796.
[48]刘志超,史晓燕,李艳根,等.镧改性粉煤灰及其脱氮除磷效果研究[J].化工新型材料,2018,46(2):205-208.
[49] Zhang Y,Yu F,Cheng W,et al. Adsorption equilibrium and kinetics of the removal of ammoniacal nitrogen by zeolite X/activated carbon composite synthesized from elutrilithe[J]. Journal of Chemistry,2017,2017(3):1-9.
[50] Chen Y Q,Tang J J,Wen-Long L I,et al. Thermal decomposition of magnesium ammonium phosphate and adsorption properties of its pyrolysis products toward ammonia nitrogen[J]. Transactions of Nonferrous Metals Society of China,2015,25(2):497-503.